Welcome to Noda Lab's Home Page
Nanomaterials & Self-Organization
Nanotechnology brings innovations to the society
widely in energy/environment, information/communication, etc.,
by adding novel functions to materials by controlling their structures
at nanometer-scale. We are trying to establish the base of materials nanotechnology.
Let us think about the future clean energy systems. For large-scale electric power generation
by solar cells, efficient use of high purity silicon is the key so that we are trying to
improve the efficiency several-ten times by making single-crystalline thin films.
Transparent electrodes are important for both solar cells (yielding electricity from light)
and displays & lightings (generating lights from electricity),
and we try to replace metal oxide semiconductors using rare-elements with carbon nanotubes or graphene.
Nanotube-silicon hybrids are promising to realize Li ion batteries
of larger capacities for (hybrid) electric vehicles.
In this way, nanotechnology can bring innovations widely
even if we use abundant carbon and silicon elements only,
and contributes to sustainable technological society.
But nanomaterials can never be made in macro-scale if we artificially manipulate atoms/molecules one-by-one.
Self-organization, i.e. spontaneous formation of materials from numerous atoms/molecules, is the key.
We are trying to fundamentally understand the processes of chemical reactions of atoms/molecules,
formation of nanostructures, and evolution of higher-order structures.
Based on the fundamental understandings with flexible thinking and idea,
we are proposing and developing novel processes for nanomaterials and their devices.
Synthesis of Carbon Nanotubes
Single-wall carbon nanotubes (SWCNTs) are a unique 1D nanomaterial quite thin ~nm and long ~mm.
Extensive research made in physics/science fields clarified
many unique properties and potential applications for them.
On the other hand, as their price (more expensive than gold) shows, their fabrication
process is still under development and their practical applications are very much limited.
Chemistry & engineering should lead the innovations for their production and manufacturing.
We have developed rapid growth process of millimeter-long SWCNTs
and are trying to realize their practical production.
Please click here for details.
- Zhongming CHEN (D3): Understanding and engineering production of submillimeter-long carbon nanotubes.
- Mai Yamaguchi (M2): Flame synthesis of single-wall CNTs.
- Ittetsu OHBA (M1): Gas-phase synthesis of CNTs using "floating-supported catalysts" from colloidal catalyst sources.
- Kosuke KAWABATA (M1): Synthesis of submillimeter-long carbon nanotubes using catalysts
by impregnation.
- Masaaki KURIYA (M1): Second-scale growth of carbon nanotubes from acetylene black for their hybridization.
- Yusuke SUGINO (M1): Gas-phase synthesis of CNTs using "floating-supported catalysts" from catalyst salt solutions.
- Noriyoshi NAKAMURA (M1): Development of arc-CVD method for continuous production of single-wall CNTs.
- Soichiro HACHIYA (B4): Production of long CNTs by fluidized-bed and separation/collection of CNTs and support particles.
|

Rapid SWCNT growth
Larger Movie.

Continuous production by fluidized bed: Movie
|
Applications of Carbon Nanotubes
CNTs have both aspects of inorganic (having high conductivity, high tensile strength, and high thermal & chemical stabilities) and organic (light-weighted, flexible, and compatible with printing processes) matters and have a unique one-dimensional nanostructure.
In collaboration with device specialists, we are developing common electrodes & wirings for flexible electronics via dispersion & printing, and secondary batteries & electrochemical capacitors via hybridization of CNT sponge with capacitive particles.
- Nu-Ri NA(D3): Formation of dense CNT arrays for electrical and thermal conduction applications .
- Hiroyuki SHIRAE (M2): Loss-free fabrication of CNT flexible electrodes & wirings.
- Misato NARUBAYASHI (M1): Hybrid electrodes of CNT-sponge and manganase oxides for electrochemical capacitors.
- Yu YOSHIHARA(M1): Creation of Cu-C hybrid materials and evaluation of their conductivity and current carrying capacity.
- Daigo KYO (B4): Hybrid electrodes of CNT-sponge and carbon nanomaterials for electrochemical capacitors.
- Keisuke HORI (B4): Electrochemical evaluation of CNT-sponge-based electrodes for lithium ion capacitors.
- Ryo YAMADA (B4): Fabrication and electrical evaluation of printed CNT patterns.
|
Graphene
Graphene is a unique 2D nanomaterial of a single atomic layer
having excellent conducting, transparent, and mechanical properties.
But their practical production method has not been developed yet.
We are developing new processes;
directly depositing graphene on substrates in order for its electronic device applications,
and producing high quality graphene at low cost in order for its applications to solar cells and touch panels.
- Asahi OHKAWA (M1): Development of practical CVD and transfer processes for graphene.
- Yuri KISHIDA(M1): Direct formation of thin-layer graphene on substrates by etching-precipitation method.
- Kohtaro YAMAGUCHI(M1): Direct formation of graphene on substrates by solid-phase process.
- Sachie AKIBA (B4): Direct fabrication and structural control of few-layer graphene on substrates by etching-precipitation method.
- Mami TAKABATAKE (B4): Conductivity enhancement of CNT and graphene by doping for electrode/wiring applications.
|
|
Silicon
Silicon is the base for the information society.
At the same time, it contributes to the renewable energy by realizing most solar cells.
Furthermore, it has a highest theoretical capacity as an anode for lithium ion batteries.
Carbon nanotubes and graphene are also expected to make a breakthrough for energy device performance.
Targeting at the contribution to the large-scale introduction of clean energy devices,
we are trying to realize large-scale and low cost production of high-performance materials
using abundant elements of carbon and silicon.
- Jungho LEE (D3): Rapid vapor deposition and electrochemical evaluation of porous thick films of silicon-based alloys for lithium secondary batteries.
- Nan FANG (M2): Rapid vapor deposition and electrochemical evaluation of porous thick films of silicon on soft current collectors for lithium secondary batteries.
- Yuhei YAMASAKI(M1): Fabrication of large-grain crystalline silicon films by rapid vapor deposition and melting-recrystallization processes.
- Shigeki AOI (B4): Fabrication of various CNT-Cu hybrid films by rapid-vapor deposition method.
- Takayuki KOWASE (B4): Gas-phase synthesis of silicon nanoparticles by evaporation method.
- Eri MURAMOTO (B4): Basic study on low-cost solar cells based on crystalline silicon films.
- Yusuke MORIKAWA (B4): Direct fabrication of silicon particle films on current collectors for lithium secondary batteries.
|

1-min-epitaxy and lift-off of Si films for solar cells

1-min deposition of porous Si films for Li ion batteries
|
Previous Ph. D. Theses
- Kei HASEGAWA, "Millimeter-scale growth of single-walled carbon nanotubes on substrates,"
Univ. Tokyo (2011).
- Hisashi SUGIME, "Clarification of catalytic growth mechanism of single-walled carbon nanotubes
and control of their synthesis," Univ. Tokyo (2010).
- Kazunori KAKEHI, "Growth of single- and multi-walled carbon nanotubes catalyzed by sputter-deposited metal nanoparticles," Univ. Tokyo (2008).
Previous Master Theses
- Masaki KOSAKA, "Direct fabrication of metal-free graphene on substrates
and its structural control," Univ. Tokyo (2014).
- Yusuke KON, "Development of fluidized-bed process for synthesis of single-wall carbon nanotubes," Univ. Tokyo (2013).
- Kosuke HIROTA, "Fabrication of large-diameter crystalline silicon thin films for solar-cells by rapid vapor deposition method," Univ. Tokyo (2013).
- Tatsuya MASUDA, "Control of crystal growth of graphene via chemical vapor deposition using copper catalysts in face-to-face layout," Univ. Tokyo (2013).
- Jun OHSHIMA, "Flame synthesis of single-wall carbon nanotubes,"
Univ. Tokyo (2011).
- Yoshikuni SATO, "Gas-phase synthesis of single-wall carbon nanotubes and their structure control," Univ. Tokyo (2011).
- Nu-Ri NA, "Low temperature growth of vertically aligned dense carbon nanotube arrays on substrates,"
Univ. Tokyo (2011).
- Kotaro SEKIGUCHI, "Instant implementation of carbon nanotube field emitters by pulse-current heating CVD," Univ. Tokyo (2011).
- Soichiro TAKANO, "Direct fabrication of metal-free graphene films on substrates," Univ. Tokyo (2011).
- Kyu-Ha LEE, "Fabrication of dense FePt nanorod arrays by separation of sputtered polycrystalline films at their grain boundaries," Univ. Tokyo (2011).
- Heunku KANG, "Fabrication of graphene from amorphous carbon by metal-induced crystallization and crystal growth mechanism," Univ. Tokyo (2011).
- Suarpa KETPREECHASAWAT, "Self-organized networks of carbon nanotubes and their transparent conducting properties (2010).
- Sang Wook PARK, "Sustainable centimeter-scale growth of carbon nanotubes," Univ. Tokyo (2010).
- Yoko ISHITSUKA, "Gas-phase synthesis of single-walled carbon nanotubes by gas-suspended catalysts and their growth mechanism," Univ. Tokyo (2010).
- Yukie TSUJI, "Structural control of polycrystalline cobalt silicide thin films," Univ. Tokyo (2010).
- Keisuke NOMURA, "Development of catalysts for low temperature growth of carbon nanotubes," Univ. Tokyo (2010).
- Takashi SHIRAI, "Low temperature growth of carbon nanotubes and their dense growth by thin-film catalysts (2009).
- F. Kanyiri MUNGAI, "Rapid epitaxial growth and lift-off process for fabrication of single-crystalline silicon thin films for solar cells," Univ. Tokyo (2009).
- Shingo MOROKUMA, "Development of Si thin film anode for Li ion secondary battery," Univ. Tokyo (2009).
- Ryuhei ITO, "Separate control of the gas-phase and catalytic reactions in catalytic CVD synthesis of carbon nanotubes," Univ. Tokyo (2008).
- Satoshi TAKASHIMA, "Understanding of Cu deposition mechanism under chlorine atmosphere and development of via-filling process," Univ. Tokyo (2008).
- Kei HASEGAWA, "Rapid growth of single-walled carbon nanotubes on substrate by thermal CVD method," Univ. Tokyo (2008).
- Hiroshi OHSHIMA, "Synthesis and characterization of amorphous silica film showing phase transition from semiconductor to insulator," Univ. Tokyo (2007).
- Yuichi KUWAHARA, "Fabrication of crystalline silicon thin films for solar cells by epitaxial lift-off method (2007).
- Hisashi SUGIME, "Combinatorial screening of catalysts and basics and control of single-walled carbon nanotube growth," Univ. Tokyo (2007).
- Azusa MORISHITA, "Grain boundary control of sputtered, magnetic FePt nanocrystalline thin films," Univ. Tokyo (2007).
Previous Bachelor Theses
- Ittetsu OHBA, "Creation of aerosol supported catalyst from colloidal solution and gas-phase synthesis of carbon nanotubes," Waseda Univ. (2014).
- Kosuke KAWABATA, "Synthesis of submillimeter-long carbon nanotubes using catalysts by impregnation," Waseda Univ. (2014).
- Yuri KISHIDA, "Direct synthesis of graphene on dielectric substrates from Co-C mixture films by etching-precipitation method," Waseda Univ. (2014).
- Masaaki KURIYA, "Hybrid formation through carbon nanotube growth on acetylene black particles and reaction control in 1-second time scale ," Waseda Univ. (2014).
- Yusuke SUGINO, "Creation of aerosol supported catalyst from catalyst salt solution and gas-phase synthesis of carbon nanotube," Waseda Univ. (2014).
- Noriyoshi NAKAMURA, "Continuous production of carbon nanotubes using arc-discharge and gaseous carbon source," Waseda Univ. (2014).
- Misato NARUBAYASHI, "Fabrication of hybrid electrodes of self-supporting carbon nanotube films with MnO2 particles for electrochemical capacitors," Waseda Univ. (2014).
- Kohtaro YAMAGUCHI, "Fabrication and structure control of graphene thin films by gas-phase and solid-phase processes," Waseda Univ. (2014).
- Yuhei YAMASAKI, "Fabrication method of crystalline silicon thin films for flexible solar cells
," Waseda Univ. (2014).
- Yu YOSHIHARA, "Fabrication of Cu-C hybrid films by sputter-deposition and evaluation of their conductivity and current-carrying capacity," Waseda Univ. (2014).
- Asahi OHKAWA, "Transfer of graphene synthesized by CVD on catalysts and repeated use of the catalysts," Waseda Univ. (2013).
- Hiroyuki SHIRAE, "Facile fabrication of flexible wirings and transparent electrodes of carbon nanotubes," Waseda Univ. (2013).
- Nan FANG, "Rapid vapor deposition of silicon-based porous films for anodes of lithium ion batteries," Waseda Univ. (2013).
- Mai YAMAGUCHI, "Flame synthesis of single-wall carbon nanotubes," Waseda Univ. (2013).
- Kosuke HIROTA, "Fabrication of single-crystalline silicon thin films for solar cells
by rapid vapor deposition and epitaxial lift-off methods," Univ. Tokyo (2011).
- Tatsuya MASUDA, "Fabrication and structural control of graphene
by chemical vapor deposition using Cu thin film catalysts," Univ. Tokyo (2011).
- Yoshikuni SATO, "Gas-phase synthesis of single-walled carbon nanotube seeds," Univ. Tokyo (2010).
- Kotaro SEKIGUCHI, "Instant implementation of carbon nanotube field emitters by pulse-current heating (2009).
- Soichiro TAKANO, "Developing a selective filling method of micro-pores," Univ. Tokyo (2009).
- Yukie TSUJI, "Understanding and controlling crystal growth of cobalt silicide thin films for electronic devices (2008).
- Keisuke NOMURA, "Low temperature growth of carbon nanotubes by function-shared catalysts," Univ. Tokyo (2008).
- Shingo MOROKUMA, "Structural change of catalyst nanoparticles during carbon nanotube growth," Univ. Tokyo (2007).
Previous versions of this page
current version
| FY2013
| FY2012